Seminars

Niklas Witt

Europe/London
S7.06

S7.06

Description

Real-space switching of local moments driven by quantum geometry in correlated graphene Heterostructures

Graphene-based multilayer systems serve as versatile platforms for exploring the interplay between electron correlation and topology, thanks to distinctive low-energy bands marked by significant quantum metric and Berry curvature from graphene’s Dirac bands. Here [1], we investigate Mott physics and local spin moments in Dirac bands hybridized with a flat band of localized orbitals in functionalized graphene. Via hybridization control, a topological transition is realized between two symmetry-distinct site-selective Mott states featuring local moments in different Wyckoff positions, with a geometrically enforced metallic state emerging in between. We find that this geometrically controlled real-space switching of local moments and associated metal-insulator physics may be realized through proximity coupling of epitaxial graphene on SiC(0001) with group IV intercalants, where the Mott state faces geometrical obstruction in the large-hybridization limit. This work shows that chemically functionalized graphene provides a correlated electron platform, very similar to the topological heavy fermions in graphene moiré systems but at significantly enhanced characteristic energy scales.

[1] N. Witt et al., arXiv:2503.03700 (to appear in Phys. Rev. Lett.)